Beilstein J. Nanotechnol.2026,17, 505–514, doi:10.3762/bjnano.17.33
-Liebknecht-Straße 24/25, 14476 Potsdam-Golm, Germany 10.3762/bjnano.17.33 Abstract This study investigates size-controlled, quantum-confined CdSe/ZnS core–shell quantum dots using core-holeclock spectroscopy in combination with post-collision interaction (PCI) line shape analysis, providing insights into
experimental approach enables the simultaneous observation of collective electronic properties and atom-specific dynamics within in a single measurement under identical sample conditions, an advance particularly valuable for complex, sensitive materials.
Keywords: core-holeclock; nanoparticles; post
surface ligands [14].
In this work, we obtain charge transfer on the atomic scale for size-dependent quantum-confined systems using core-holeclock (CHC) spectroscopy. We further expand the well-established CHC approach by the aspect of detecting the internal continuum states within the size-controlled
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Figure 1:
S KL2,3L2,3 resonant Auger measurements of core–shell nanoparticles (core: 3.5 nm CdSe, shell: 7 do...
Beilstein J. Nanotechnol.2020,11, 1663–1684, doi:10.3762/bjnano.11.149
states and the dynamical CT in the excited state can be probed by photoemission spectroscopy (PES). In particular, coreholeclock spectroscopy has been used to measure the time constant of dynamical CT in the valence band states as a function of the lifetime of the core hole, which is typically of the
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Figure 1:
(a) Schematic diagram of the radiative and non-radiative decay processes of an optical excitation o...