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1 article(s) from Jiang, Xuefeng

Recent advances in controllable/divergent synthesis

Jilei Cao,
Leiyang Bai and
Xuefeng Jiang

Beilstein J. Org. Chem. 2025, 21, 890–914, doi:10.3762/bjoc.21.73

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Graphical Abstract

Scheme 1: Ligand-controlled regiodivergent C1 insertion into arynes [19].

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Scheme 2: Ligand effect in homogenous gold catalysis enabling regiodivergent π-bond-activated cyclization [20].

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Scheme 3: Ligand-controlled palladium(II)-catalyzed regiodivergent carbonylation of alkynes [21].

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Scheme 4: Catalyst-controlled annulations of strained cyclic allenes with π-allyl palladium complexes and pro...

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Scheme 5: Ring expansion of benzosilacyclobutenes with alkynes [23].

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Scheme 6: Photoinduced regiodivergent and enantioselective cross-coupling [24].

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Scheme 7: Catalyst-controlled regiodivergent and enantioselective formal hydroamination of N,N-disubstituted ...

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Scheme 8: Catalyst-tuned regio- and enantioselective C(sp³)–C(sp³) coupling [31].

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Scheme 9: Catalyst-controlled annulations of bicyclo[1.1.0]butanes with vinyl azides [32].

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Scheme 10: Solvent-driven reversible macrocycle-to-macrocycle interconversion [39].

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Scheme 11: Unexpected solvent-dependent reactivity of cyclic diazo imides and mechanism [40].

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Scheme 12: Palladium-catalyzed annulation of prochiral N-arylphosphonamides with aromatic iodides [41].

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Scheme 13: Time-dependent enantiodivergent synthesis [42].

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Scheme 14: Time-controlled palladium-catalyzed divergent synthesis of silacycles via C–H activation [43].

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Scheme 15: Proposed mechanism for the time-controlled palladium-catalyzed divergent synthesis of silacycles [43].

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Scheme 16: Metal-free temperature-controlled regiodivergent borylative cyclizations of enynes [45].

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Scheme 17: Nickel-catalyzed switchable site-selective alkene hydroalkylation by temperature regulation [46].

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Scheme 18: Copper-catalyzed decarboxylative amination/hydroamination sequence [48].

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Scheme 19: Proposed mechanism of copper-catalyzed decarboxylative amination/hydroamination sequence [48].

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Scheme 20: Enantioselective chemodivergent three-component radical tandem reactions [49].

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Scheme 21: Substrate-controlled synthesis of indoles and 3H-indoles [52].

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Scheme 22: Controlled mono- and double methylene insertions into nitrogen–boron bonds [53].

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Scheme 23: Copper-catalyzed substrate-controlled carbonylative synthesis of α-keto amides and amides [54].

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Scheme 24: Divergent sulfur(VI) fluoride exchange linkage of sulfonimidoyl fluorides and alkynes [55].

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Scheme 25: Modular and divergent syntheses of protoberberine and protonitidine alkaloids [56].

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Review

Published 07 May 2025

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