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2 article(s) from Yu, Bing

Recent advances in amidyl radical-mediated photocatalytic direct intermolecular hydrogen atom transfer

Hao-Sen Wang,
Lin Li,
Xin Chen,
Jian-Li Wu,
Kai Sun,
Xiao-Lan Chen,
Ling-Bo Qu and
Bing Yu

Beilstein J. Org. Chem. 2025, 21, 1306–1323, doi:10.3762/bjoc.21.100

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Graphical Abstract

Figure 1: (a) BDE of C–H. (b) Direct functionalization of C–H catalyzed by transition-metal. (c) Direct funct...

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Figure 2: (a) Amidyl radical-enabled hydrogen atom transfer. (b) Substituent effects to amidyl radical proper...

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Figure 3: Representative photocatalysts discussed in this review.

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Scheme 1: Alkylation of C(sp³)–H catalyzed by amidyl radical under visible light.

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Scheme 2: Direct heteroarylation of C(sp³)–H catalyzed by amidyl radical under visible light.

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Scheme 3: Alkylation of C(sp³)–H catalyzed by amidyl radical and metal-free photocatalyst under visible light....

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Scheme 4: Alkylation of C(sp³)–H, Si–H, and Ge–H catalyzed by amidyl radical under visible light.

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Scheme 5: Direct heteroarylation of C(sp³)–H catalyzed by synergistic promotion of amidyl radical and photoca...

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Scheme 6: Direct B–H functionalization of icosahedral carboranes catalyzed by amidyl radical under visible li...

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Scheme 7: Nucleophilic amination of C(sp³)–H enabled by amidyl radical under visible light.

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Scheme 8: Direct heteroarylation of C(sp³)–H and C(sp³)–H without the presence of strong bases, acids, or oxi...

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Scheme 9: Xanthylation of C(sp³)–H addressed by amidyl radical under visible light.

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Scheme 10: Xanthylation of C(sp³)–H in polyolefins addressed by amidyl radical under visible light.

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Scheme 11: Site-selective C(sp³)–H bromination implemented by amidyl radical under visible light.

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Scheme 12: Site-selective chlorination of C(sp³)–H in natural products implemented by amidyl radical under vis...

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Scheme 13: Alkylation of C(sp³)–H catalyzed by amidyl radical photocatalyst under visible light.

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Album

Review

Published 27 Jun 2025

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Synthesis of β-ketophosphonates through aerobic copper(II)-mediated phosphorylation of enol acetates

Alexander S. Budnikov,
Igor B. Krylov,
Fedor K. Monin,
Valentina M. Merkulova,
Alexey I. Ilovaisky,
Liu Yan,
Bing Yu and
Alexander O. Terent’ev

Beilstein J. Org. Chem. 2025, 21, 1192–1200, doi:10.3762/bjoc.21.96

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Scheme 1: Recent approaches for the synthesis of β-ketophosphonates by the oxyphosphorylation of unsaturated ...

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Scheme 2: The scope of the discovered copper(II)-mediated phosphorylation of enol acetates.

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Scheme 3: Gram-scale synthesis of 3a.

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Scheme 4: Control experiments.

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Scheme 5: Proposed mechanism for copper(II) mediated phosphorylation of enol acetates.

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Full Research Paper

Published 20 Jun 2025

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